Highly (002) textured Pb(ScTa)(subscript 1-x)Ti(subscript x)O3 (PSTT) (with composition x=0-0.3) thin films were deposited using metal-organic chemical vapor deposition (MOCVD) technique at temperature ranging from 600℃ to 685℃. Dielectric properties of these PSTT thin films showed strong dependency on the growth temperature and PT content. Ti addition acted as a ”Curie” temperature shifter, moving T(subscript max) from -10 to 120℃ with the dielectric constant peak value increasing from 1397 to 1992 (measured at 1 kHz) when composition x went from 0 to 0.3. Loss tangent values were generally below 0.025. For PSTT thin films with composition near its morphotropic boundary (x=0.3), the room temperature dielectric constants increased from 980 to around 1600 as the growth temperature increased from 650 to 685℃. In addition, the dielectric dispersion behaviors of films grown at different temperatures were compared.