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Fine Mode Aerosol Optical Properties Related to Cloud and Fog Processing over a Cluster of Cities in Northeast China

並列摘要


Fine mode aerosol optical properties were retrieved from sunphotometer measurements, carried out in Shenyang, Anshan, Benxi, and Fushun in Northeast China from 2009-2013. Accumulation mode aerosol size distribution retrievals were investigated for specific situations involving extensive cloud processing during fog or haze. Large fine mode median radii (≥0.20 μm) frequently occurred at the four sites in July. At other times, as aerosol optical depths increased so did the fine mode median radii, reaching 0.30-0.40 μm. This was possibly due to aerosol humidification during cloud processing. Instances of large (~1.50) Alpha curvature at the sites also may be associated with cloud processing. When single scattering albedos were ≥ 0.90, the radii distributions were centered round 0.30-0.40 μm at all at sites except Benxi, perhaps due to non-absorbing material from aerosol/cloud interactions. Case studies of size distribution retrievals at each of the four sites showed that large accumulation mode radii (0.40-0.50 μm) may be linked to cloud processing.

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