Residential Biomass Burning Emissions over Northwestern Himalayan Region of India: Chemical Characterization and Budget Estimation

Mohit Saxena ； Sudhir Kumar Sharma ； Nidhi Tomar ； Humaira Ghayas ； Avirup Sen ； Rohtash Singh Garhwal ； Naresh Chandra Gupta ； Tuhin Kumar Mandal

《Aerosol and Air Quality Research》 16卷3期 (2016/03) Pp. 504-518

https://doi.org/10.4209/aaqr.2015.04.0237

並列摘要

In the present study, we have determined the emission factors (EF) and estimated the emission of particulate matter (PM), organic carbon (OC), elemental carbon (EC), polycyclic aromatic hydrocarbons (PAHs), water soluble inorganic constituents (WSIC) and trace gases such as SO_2, NO and NO_2 from the combustion of biomass fuels (FW: fuel wood and DC: dung cake) used in rural sectors for cooking over Himachal Pradesh (HP), representing the Northwestern Himalayan region of India. The average EFs of PM estimated from FW and DC were 3.44 ± 2.38 and 11.43 ± 1.13 g kg^(-1), respectively. OC and EC emission ranged from 0.106 to 3.55 g kg^(-1) and 0.07 to 0.90 g kg–1, respectively for variety of biomass fuels. Total emission of PAHs from DC (44.37 mg kg^(-1)) and FW (43.25 mg kg^(-1)) noted in this study was almost similar. Similarly, the average EFs of NO_x from FW and DC were 0.59 ± 0.49 g kg^(-1) and 0.34 ± 0.18 g kg^(-1), respectively. FWs have comparatively higher SO_2 emission (average: 0.43 ± 0.38 g kg^(-1)) than from DC (average: 0.23 ± 0.15 g kg^(-1)). Among anionic inorganic constituents emitted from FW, maximum EF was noted for Cl- (0.30 ± 0.26 g kg^(-1)). Similarly for cations, highest EF was noted of K+ (0.20 ± 0.09 g kg^(-1)). Ca^(2+) and Na+ were the major cationic species identified in plumes of DC burning. Utilizing total annual consumption of biomass fuels and EFs of particulates and trace gases determined in the present study over HP and in the past study (Saud et al., 2011, 2012) over Uttarakhand, budget estimates of PM, OC, EC, TC, PAHs, SO_2 and NO_x have been determined over the Northwestern Himalayan region. Total annual emission estimated over Northwestern Himalayan region are as: PM (18.32 ± 9.53 Gg), OC (4.38 ± 2.31 Gg), EC (1.39 ± 0.55 Gg) and trace gases (SO2: 1.47 ± 1.0 Gg; NOx: 1.77 ± 1.31 Gg).

並列關鍵字

Particulate matter ； Trace gases ； Emission factor ； Budget estimation ； Northwestern Himalayan region