- 期刊
- OpenAccess
A Long-lasting Winter Haze Episode in Xiangyang, Central China: Pollution Characteristics, Chemical Composition, and Health Risk Assessment
摘要
This study investigated the characteristics and chemical composition of PM_(2.5) during a long-lasting winter haze episode (Jan. 13-24, 2018) in Xiangyang of central China. The average daily concentration of the PM_(2.5) equaled 169.29 ± 56.98 μg m^(-3), with water-soluble inorganic ions (WSIIs), organic carbon (OC), elemental carbon (EC), and trace elements accounting for 111.45 ± 44.62, 20.74 ± 6.79, 6.48 ± 1.79, and 10.53 ± 3.84 μg m^(-3), respectively. The OC/EC ratios indicated mixed contributions from intensive traffic emission and secondary formation, and the estimated concentrations for the primary organic carbon (POC) and the secondary organic carbon (SOC) increased with the level of pollution. POC dominated the OC during mild and moderate pollution, whereas SOC dominated it during severe pollution. A strong positive correlation was found between the enrichment factor (EF) and geo-accumulation index (I_(Geo)) values, which were used to assess the contamination level of PM_(2.5)-bound metal(loid)s. A health risk assessment, which was conducted to examine the non-carcinogenic and carcinogenic risks of the PM_(2.5)-bound metal(loid)s, found that As, Cr, Pb, and Sb posed potential non-carcinogenic risks to both children and adults and that two of these elements, As and Pb, also posed potential carcinogenic risks. The total non-carcinogenic and carcinogenic risks from the PM_(2.5)-bound metal(loid)s were slightly higher for adults (3.07 × 10^3 and 3.78 × 10^(-3)) than children (2.71 × 10^3 and 2.99 × 10^(-3)) and depended on the concentrations of the metal(loid)s rather than the level of pollution. Thus, the public and the government should implement appropriate measures to mitigate the health risks posed by PM_(2.5)-bound metal(loid)s during winter haze episodes in Xiangyang.
延伸閱讀
- Du, C. L., Liu, S. Y., Yu, X., Li, X. M., Chen, C., Peng, Y., Dong, Y., Dong, Z. P., & Wang, F. Q. (2013). Urban Boundary Layer Height Characteristics and Relationship with Particulate Matter Mass Concentrations in Xi'an, Central China. Aerosol and Air Quality Research, 13(5), 1598-1607. https://doi.org/10.4209/aaqr.2012.10.0274
- Wang, H. L., Zhu, B., Shen, L. J., Xu, H. H., An, J. L., Pan, C., Li, Y., & Liu, D. Y. (2016). Regional Characteristics of Air Pollutants during Heavy Haze Events in the Yangtze River Delta, China. Aerosol and Air Quality Research, 16(9), 2159-2171. https://doi.org/10.4209/aaqr.2015.09.0551
- Xu, Q. P., Wang, J. Z., Liu, J. Q., & Peng, S. C. (2017). Particulate Size Distribution and Sources Evaluation of n-Alkanes during Long-Term Haze Episode around Chaohu Lake, Eastern China. Aerosol and Air Quality Research, 17(8), 1975-1984. https://doi.org/10.4209/aaqr.2017.05.0189
- Gao, Q., Yan, Y., Li, R., Xu, Y., Niu, Y., Liu, C., Xie, K., Chang, Z., Hu, D., Li, Z., & Peng, L. (2020). Characteristics of Volatile Organic Compounds during Different Pollution Periods in Winter in Yuncheng, a Typical City in North China. Aerosol and Air Quality Research, 20(1), 97-107+ap1-4. https://doi.org/10.4209/aaqr.2019.08.0402
- Chen, F., Zhang, X., Zhu, X., Zhang, H., Gao, J., & Hopke, P. K. (2017). Chemical Characteristics of PM_(2.5) during a 2016 Winter Haze Episode in Shijiazhuang, China. Aerosol and Air Quality Research, 17(2), 368-380(i-i). https://www.airitilibrary.com/Article/Detail?DocID=16808584-201702-201702150008-201702150008-368-380(i-i)