The researcher who is a psychology doctoral student and a writer attempts to describe the literary psychology by comparing the psychological imagination and writing experience with his learning in psychology class. After four stages of research, the researcher realizes the literary psychology has substantive connotation through invoking psychobiography. There are two ways to express the substantive connotation, one is Western Psychobiography, and the other is Chinese Philosophy. In conclusion, psychobiography is not only for Western but for Chinese and Literature. People in psychobiography is recognized a touching, meaningful, historical and social literature, also a creative art.