In this study, observations of inner radiation belt recorded by Relativistic Proton Spectrometer onboard the Van Allen Probes Mission are adopted to explore the spatial and temporal distributions of protons of energies higher than about 60 megaelectronvolts in the inner radiation belt. The analysis focuses on the periods during large Solar Proton Events with intensities larger than 1000 particle flux unit from the year of 2013 to 2017. The results show that the inner radiation belt could expand and the energetic protons could penetrate deeply toward the Earth when large Solar Proton Events occurred. Moreover, the results also show that large Solar Proton Events may be a contributing factor to induce geomagnetic storms. The results of this study could also be referred for designing of satellite orbits and radiation shielding.