The surface magneto-optical Kerr effect measurement in high vacuum was performed with a millisecond-pulsed magnetic field, which is generated from the controlled discharge of capacitors to the coils. The theoretical simulation is used to obtain the strong and uniform pulsed magnetic field. Compared with the conventional electromagnet, pulsed magnetic field is faster. The maximum field strength can be improved by increasing the charging voltage. A nickel film on the SiO2 is used as the test sample, and its magnetic hysteresis loop was successfully obtained. The magnetic coercive, remanence, and hysteresis curve characteristics of the magnetic film were observed. The results were consistent with the measurement methods of other periodicals. Verify the accuracy of this device measurement. This technique can be applied to the study of the dynamic magnetic properties in the future.