利用還原氧化石墨烯及奈米銀線製備高性能可撓曲透明導電膜之研究

賴怡廷

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利用還原氧化石墨烯及奈米銀線製備高性能可撓曲透明導電膜之研究

High performance flexible transparent conductive films based on reduced graphene oxides and silver nanowires

賴怡廷 , Masters　　Advisor：戴念華　　

繁體中文

奈米銀線；還原氧化石墨烯； p型摻雜效應；透明導電軟板；單一製程； silver nanowires ； reduced graphene oxide ； p-type doping ； flexible transparent conductive films ； one-step process

Abstract │ Reference (81) │ Altmetrics

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This work demonstrates an one-step process to synthesize uniformly dispersed hybrid nanomaterial containing silver nanowires (AgNWs) and p-type reduced graphene (p-rGO). The hybrid nanomaterial was coated onto a polyethylene terephthalate (PET) substrate to prepare high performance flexible transparent conductive films (TCFs). The p-rGO plays the role of bridging discrete AgNWs, providing more electron holes, and lowering the resistance of the contacted AgNWs, which enhances the electrical conductivity without sacrificing too much transparence of the TCFs. In addition, the p-rGO also improves the adhesion between AgNWs and substrate by covering the AgNWs on substrate tightly. The study shows that coating of the hybrid nanomaterials on the PET substrate demonstrates exceptional optoelectronic properties with a transmittance of 94.68% (at a wavelength of 550 nm) and a sheet resistance of 25.0 ohm/sq. Furthermore, no significant variation in electric resistance can be detected even though the film was subjected to a bend loading with a radius of curvature of 5.0 mm or the film was loaded with a reciprocal tension or compression for 1000 cycles. The study shows that the fabricated flexible TCFs have the potential to replace indium tin oxide film in the optoelectronic industry.

Reference ( 81 ) 〈TOP〉

1. Lien, S. Y. Characterization and optimization of ITO thin films for application in heterojunction silicon solar cells. Thin Solid Films 2010, 518, S10-S13.
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2. Suzuki, Y.; Niino, F.; Katoh, K. Low-resistivity ITO films by dc arc discharge ion plating for high duty LCDs. Journal of Non-Crystalline Solids 1997, 218, 30-34.
連結：
3. Tak, Y.-H.; Kim, K. B.; Park, H. G.; Lee, K. H.; Lee, J. R. Criteria for ITO (indium–tin-oxide) thin film as the bottom electrode of an organic light emitting diode. Thin Solid Films 2002, 411, 12-16.
連結：
4. Tseng, S. F.; Hsiao, W.-T.; Huang, K. C.; Chiang, D.; Chen, M. F.; Chou, C. P. Laser scribing of indium tin oxide (ITO) thin films deposited on various substrates for touch panels. Applied Surface Science 2010, 257, 1487-1494.
連結：
5. Hanson, E. L.; Guo, J.; Koch, N.; Schwartz, J.; Bernasek, S. L. Advanced surface modification of indium tin oxide for improved charge injection in organic devices. Journal of the American Chemical Society 2005, 127, 10058-10062.
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