具方向性鍵結的二氧化鈦在染料敏化太陽能電池之應用

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具方向性鍵結的二氧化鈦在染料敏化太陽能電池之應用

Dye-Sensitized Solar Cells Based on an Oriented Attachment Anatase TiO2 Secondary Structure

廖俊侯 , Masters　　Advisor：郭炳林　　

繁體中文

方向性鍵結；二氧化鈦；紅汞；染料敏化太陽能電池； DSSC ； oriented attachment ； TiO2 ； Mercurochrome

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In this study, a novel surfactant TEOA-C10 was synthesized to prepare anatase titania nanoparticles with secondary structures by a surfactant-assisted self-assembling process. The crystal lattice planes of the second structure were aligned with each other due to the “oriented attachment” mechanism, which is expected to increase the rate of electron transfer through the highly crystallized second structure. The grain size and secondary structure were controlled by changing the mole ratio of TEOA-C10 to titanium precursor and the temperature of the hydrothermal via control of the grain size, second structure, and thermal stability for the TiO2 second structure. A single-crystalline anatase photoelectrode adsorbed mercurochrome dye about 4~5 times higher as compared to P25.
    A light-to-electricity conversion yield of 1.31% was achieved by applying the titania nanomaterials with 2 micrometer thin film, and it can increase to 1.68~1.69%, if using double layer photoelectrode made by anatase titania nanoparticle and P25. When the dye was changed from mercurochrome to N719, double layer still can improve the light-to-electricity conversion efficiency from 3.91% to 4.57%.

Reference ( 64 ) 〈TOP〉

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連結：
4. M. Adachi, Y. Murata, J. Takao, J. Jiu, M. Sakamoto, and F. Wang, "Highly Efficient Dye-Sensitized Solar Cells with a Titania Thin-Film Electrode Composed of a Network Structure of Single-Crystal-like TiO2 Nanowires Made by the "Oriented Attachment" Mechanism," J. Am. Chem. Soc. 126 (45), 14943-14949 (2004).
連結：
7. L. Thomas, M. Paul, and H. Arnim, "Surface chemistry of colloidal silver: surface plasmon damping by chemisorbed iodide, hydrosulfide (SH-), and phenylthiolate " J. Phys. Chem. 97 (3), 679-682 (1993).
連結：
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連結：
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連結：

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