The purposes of this study were to explore the improvement effect of urban park development for particle air pollutants in Taipei and Kaohsiung cities. The study areas were the 500m effective monitoring radius of air quality monitoring stations in Taipei and Kaohsiung cities. We investigated the areas of urban park and industry park, roadsides trees, traffic flow, and particulate matters quality (Dust-fall, TSP, PM10). Then we used the regression analysis method to analyze the improvement effect of urban parks and roadsides trees for particle air pollutants. The results suggest that there is a significant effect between the urban parks or roadsides trees and Dust-fall and TSP. It shows that the more urban parks or roadsides trees, the less concentration of Dust-fall and TSP. It concludes that the governments should development more urban parks or roadsides trees near the industry areas and the main roads for improving urban environmental quality.