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The Impacts of Emission Control and Regional Transport on PM_(2.5) Ions and Carbon Components in Nanjing during the 2014 Nanjing Youth Olympic Games
摘要
Highly time-resolved measurements of water soluble ions, organic and elemental carbon concentrations in the particle diameter size range D_p ＜ 2.5 μm (PM_(2.5)) were performed at a downwind urban site in Nanjing in the western part of the Yangtze River Delta (YRD) in eastern China during the 2014 Youth Olympic Games (YOG). In this study, we discuss the impacts of emission control in Nanjing and the surrounding areas during the YOG and regional/long-range transport on PM_(2.5) pollution in Nanjing. The average concentrations of NO_3^-, SO_4^(2-), NH_4^+ were 12.1 ± 9.9, 16.5 ± 9.2, 9.0 ± 5.4 μg m^(-3) during the YOG, and increased 34.3%, 53.7%, 43.9% after the YOG, respectively. The control of construction or on-road soil dust and control of industry led to the decrease of Ca^(2+) concentration by 55% and SO_2 concentration by 46%. However, SO_4^(2-) concentrations remained at relatively high levels, suggesting a significant impact of regional pollution to secondary fine particles in Nanjing. Strong correlations between OC and EC were observed during and after the YOG. A higher percentage (41%) of secondary organic carbon in Nanjing during the YOG periods was consistent with high potential photochemistry and low contributions from coal combustion. Lagrangian dispersion modelling results proved that the city clusters along the Nanjing and Shanghai axis were the major source region for high PM_(2.5) pollution in upwind Nanjing. This work shows that short-term strict control measures could improve the air quality, especially that affected by the primary pollutants; however, regional collaborative control strategy across administrative borders in the YRD is needed for a substantial improvement of air quality.
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延伸閱讀
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