- 期刊
- OpenAccess
Assessment of the Integrated Personal Exposure to Particulate Emissions in Urban Micro-environments: A Pilot Study
摘要
City dwellers' personal exposure to PM is influenced by numerous daily activities in multiple indoor and outdoor micro-environments (MEs). This study assessed the integrated personal exposure to PM across urban MEs together with the recording individual time-activity patterns. We evaluated simultaneously the exposure to PM_(2.5), black carbon (BC), and ultrafine particles (UFPs) in the Central Business District (CBD) area of Singapore. In addition, we quantified the lung-deposited surface area (LDSA) concentration, which is an indicator of the potential health impacts of UFPs. The field study was conducted over a 7-km walking route to identify air pollution hotspots. Subsequently, the personal exposure to PM_(2.5), BC, and UFPs was measured at five selected hotspots for 1 hour each and across indoor and outdoor MEs during diverse daily human activities for 24 hours. The PM concentrations were found to vary considerably in both space and time in the CBD area. During the 1-hour personal exposure measurement, extremely high concentrations of PM_(2.5) (215 ± 129.5 μg m^(-3) and 36.4 ± 12.5 μg m^(-3)) and BC (20.9 ± 10.4 μg m^(-3) and 18.1 ± 12.0 μg m^(-3)) were observed at a temple and a bus stop, and elevated UFP number concentrations (320.8 ± 131.1 × 10^3 # cm^(-3)) and high LDSA concentrations (564.6 ± 276.5 μg^2 cm^(-3)) were measured at a food court. The estimated potential health risk suggests that the continued inhalation of large amounts of PM_(2.5) emitted from combustion sources is likely to lead to adverse long-term health effects among the exposed individuals. Overall, we provide insight into an individual's total exposure to PM based on time-activity patterns. The results of this work form a scientific basis for developing air pollution control measures to mitigate personal exposure to PM on a city scale.
延伸閱讀
- Mohammadyan, M., Larimi, A. A., Etemadinejad, S., Latif, M. T., Heibati, B., Yetilmezsoy, K., Wahab, S. A. A., & Dadvand, P. (2017). Particulate Air Pollution at Schools: Indoor-Outdoor Relationship and Determinants of Indoor Concentrations. Aerosol and Air Quality Research, 17(3), 857-864(i-i). https://www.airitilibrary.com/Article/Detail?DocID=16808584-201703-201703030015-201703030015-857-864(i-i)
- Harpale, V. M., Ralegankar, S. D., Jadhav, D. B., & Dhole, S. D. (2006). Chemical Identification of Urban Air Particulates in the Environment of Pune City (India) by Raman Spectroscopy. Aerosol and Air Quality Research, 6(3), 295-304. https://www.airitilibrary.com/Article/Detail?DocID=16808584-200609-6-3-295-304-a
- Ashworth, D. C., Fuller, G. W., Toledano, M. B., Font, A., Elliott, P., Hansell, A. L., & Hoogh, K. D. (2013). Comparative Assessment of Particulate Air Pollution Exposure from Municipal Solid Waste Incinerator Emissions. Journal of Environmental and Public Health, 2013(), 292-304. https://doi.org/10.1155/2013/560342
- Beal, A., Bufato, C. A., Almeida, D. S. D., Squizzato, R., Zemiani, A., Vernilo, N., Batista, C. E., Salvador, G., Borges, D. L., Solci, M. C., Silva, A. F. D., Martins, J. A., & Martins, L. D. (2017). Inorganic Chemical Composition of Fine Particulates in Medium-Sized Urban Areas: A Case Study of Brazilian Cities. Aerosol and Air Quality Research, 17(4), 920-932+ap1-1. https://doi.org/10.4209/aaqr.2016.07.0317
- Kuula, J., Kuuluvainen, H., Rönkkö, T., Niemi, J. V., Saukko, E., Portin, H., Aurela, M., Saarikoski, S., Rostedt, A., Hillamo, R., & Timonen, H. (2019). Applicability of Optical and Diffusion Charging-Based Particulate Matter Sensors to Urban Air Quality Measurements. Aerosol and Air Quality Research, 19(5), 1024-1039+ap1-7. https://doi.org/10.4209/aaqr.2018.04.0143