Vapor-deposited nanostructured silver film was fabricated by using oblique angle depositon technique. When a silver NRA is illuminated by s-polarized and p-polarized light, the transverse plasmon and the longitudinal plasmon modes are excited, respectively. The anisotropic transmission and reflection coefficients of the silver film were measured by walk-off interferometer. The equivalent refractive indices of the silver film were demonstrated to be negative over the visible regime.